RESUMO
We consider two-species random sequential adsorption (RSA) in which species A and B adsorb randomly on a lattice with the restriction that opposite species cannot occupy nearest-neighbor sites. When the probability x_{A} of choosing an A particle for an adsorption trial reaches a critical value 0.626441(1), the A species percolates and/or the blocked sites X (those with at least one A and one B nearest neighbor) percolate. Analysis of the size-distribution exponent τ, the wrapping probabilities, and the excess cluster number shows that the percolation transition is consistent with that of ordinary percolation. We obtain an exact result for the low x_{B}=1-x_{A} jamming behavior: θ_{A}=1-x_{B}+b_{2}x_{B}^{2}+O(x_{B}^{3}), θ_{B}=x_{B}/(z+1)+O(x_{B}^{2}) for a z-coordinated lattice, where θ_{A} and θ_{B} are, respectively, the saturation coverages of species A and B. We also show how differences between wrapping probabilities of A and X clusters, as well as differences in the number of A and X clusters, can be used to find the percolation transition point accurately.
RESUMO
Multiple-spin coupling is a key tool for investigating magnetic quantum systems. In particular, models with four-spin interactions became of great interest since they have been applied to describe material properties such as superconductivity. In this framework, the dynamics of the spin-1/2 Ising two-leg ladder with four-spin plaquette interaction in a transverse field is investigated. By means of the recurrence relations method, the first four recurrants are determined exactly for the general model, while five exact recurrants are calculated for two particular models. In all cases, higher-order recurrants are computed through extrapolation to obtain time-dependent autocorrelation functions and spectral densities in the long-time regime and infinite-temperature limit. It is found that the relaxation functions decay slower than the expected behavior of the one-dimensional transverse Ising model. The spectral lines, characterized by a Lorentzian behavior in the central body and a Gaussian shape in the tails, display exchange narrowing as the coupling intensities increase.
RESUMO
Advanced chain-growth computer simulation methodologies have been employed for a systematic statistical analysis of the critical behavior of a polymer adsorbing at a substrate. We use finite-size scaling techniques to investigate the solvent-quality dependence of critical exponents, critical temperature, and the structure of the phase diagram. Our study covers all solvent effects from the limit of super-self-avoiding walks, characterized by effective monomer-monomer repulsion, to poor solvent conditions that enable the formation of compact polymer structures. The results significantly benefit from taking into account corrections to scaling.
RESUMO
By means of contact-density chain-growth simulations of a simple coarse-grained lattice model for a polymer grafted at a solid homogeneous substrate, we investigate the complementary behavior of the numbers of surface-monomer and monomer-monomer contacts under various solvent and thermal conditions. This pair of contact numbers represents an appropriate set of order parameters that enables the distinct discrimination of significantly different compact phases of polymer adsorption. Depending on the transition scenario, these order parameters can interlock in perfect cooperation. The analysis helps understand the transitions from compact filmlike adsorbed polymer conformations into layered morphologies and dissolved adsorbed structures, respectively, in more detail.
